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Reaction of imidazole derivatives with trifluoromethylated arylacetylenes
The nucleophilic addition of imidazole derivatives to trifluoromethylated acetylenes was studied. Unpredictable regioselectivity of the reaction was observed to yield both beta- and alpha-addition products. The reaction is 100% stereoselective to give the corresponding adducts as a Z-isomers only. The observed regioselectivity is discussed in terms of polarization of triple bond using experimental and calculated data. (C) 2016 Elsevier B.V. All rights reserved.
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